Résumé
Volatile organic compounds (VOCs) have direct influences on air quality and climate. They indeed play a key role in atmospheric chemistry as precursors of secondary pollutants, such as ozone (O3) and secondary organic aerosols (SOA). In this respect, long-term datasets of in situ atmospheric measurements are crucial for characterizing the variability of atmospheric chemical composition, its sources, and trends. The ongoing establishment of the Aerosols, Cloud, and Trace gases Research InfraStructure (ACTRIS) allows implementation of the collection and provision of such high-quality datasets. In this context, online and continuous measurements of O3, nitrogen oxides (NOx), and aerosols have been carried out since 2012 at the SIRTA (Site Instrumental de Recherche par Télédétection Atmosphérique) observatory, located in the Paris region, France. Within the last decade, VOC measurements were conducted offline at SIRTA, until the implementation of real-time monitoring which started in January 2020 using a proton-transfer-reaction quadrupole mass spectrometer (PTR-Q-MS).The dataset acquired during the first 2 years of online VOC measurements provides insights into their seasonal and diurnal variabilities. The additional long-term datasets obtained from co-located measurements (NOx, aerosol physical and chemical properties, meteorological parameters) are used to better characterize the atmospheric conditions and to further interpret the obtained results. Results also include insights into VOC main sources and the influence of meteorological conditions and air mass origin on their levels in the Paris region. Due to the COVID-19 pandemic, the year 2020 notably saw a quasi-total lockdown in France in spring and a lighter one in autumn. Therefore, the focus is placed on the impact of these lockdowns on the VOC variability and sources. A change in the behaviour of VOC markers for anthropogenic sources was observed during the first lockdown, reflecting a change in human activities. A comparison with gas chromatography data from the Paris city centre consolidates the regional representativity of the SIRTA station for benzene, while differences are observed for shorter-lived compounds with a notable impact of their local sources. This dataset could be further used as input for atmospheric models and can be found at 10.14768/f8c46735-e6c3-45e2-8f6f-26c6d67c4723 (Simon et al., 2022a).
Résumé
Understanding near-surface atmospheric behavior in the tropics is imperative given the role of tropical energy fluxes in Earth’s climate cycles, but this area is complicated by a land–atmosphere interaction that includes rugged to-pography, seasonal weather drivers, and frequent environmental disturbances. This study examines variation in nearsurface atmospheric behaviors in northeastern Puerto Rico using a synthesis of data from lowland and montane locations under different land covers (forest, urban, and rural) during 2008–21, when a severe drought, large hurricanes (Irma and Maria), and the COVID-19 mobility-reducing lockdown occurred. Ceilometer, weather, air quality, radiosonde, and satellite data were analyzed for annual patterns and monthly time series of data and data correlations. The results showed a system that is strongly dominated by easterly trade winds transmitting regional oceanic patterns over terrain. Environmental disturbances affected land–atmosphere interaction for short time periods after events. Events that reduce the land signature (reducing greenness: e.g., drought and hurricanes, or reducing land pollution: e.g., COVID-19 lockdown) were evidenced to strengthen the transmission of the oceanic pattern. The most variation in near-surface atmospheric behavior was seen in the mountainous areas that were influenced by both factors: trade winds, and terrain-induced orographic lifting. As an exception to the rest of the near-surface atmospheric behavior, pollutants other than ozone did not correlate positively or negatively with stronger trade winds at all sites across the region. Instead, these pollutants were hypothesized to be more anthropogenically influenced. Once COVID-19 lockdown had persisted for 3 months, urban pollution decreased and cloud base may have increased. © 2022, American Meteorological Society. All rights reserved.
Résumé
COVID-19 lockdown resulted in the revival of the environment due to reduced emissions of various pollutants globally. In particular, aerosols, NOx and SO2 showed significant reductions at most places. However, the greenhouse gases are not necessarily following this reduction everywhere. In most areas, a decrease in NOx increases methane (CH4) concentration by enhancing the lifetime, but also results in decreased concentrations with reduced emissions. Analyzing the atmospheric CH4 variations during the COVID-19 lockdown over India is crucial as India is one of the regions with high seasonal variability of CH4. The present study has analyzed the tropospheric CH4 trends over India during the pre-monsoon season (March-May) for 2003-2021 using AIRS data. The study analyzed the lockdown variations (24 March-31 May) of tropospheric CH4 over India with the same period of 2019 and 2021 using TROPOMI to find the changes in CH4 concentrations over different regions of India due to lockdown. Our results capture the undeviating north (low)-south (high) gradient in the CH4 concentration with anticipated regional intensifications, likely, in the eastern and western coastal regions, with more comprehensive details than it ever has been presented before.
Résumé
Like several countries, Spain experienced a multi wave pattern of COVID-19 pandemic over more than one year period, between spring 2020 and spring 2021. The transmission of SARS-CoV-2 pandemics is a multi-factorial process involving among other factors outdoor environmental variables and viral inactivation.This study aims to quantify the impact of climate and air pollution factors seasonality on incidence and severity of COVID-19 disease waves in Madrid metropolitan region in Spain. We employed descriptive statistics and Spearman rank correlation tests for analysis of daily in-situ and geospatial time-series of air quality and climate data to investigate the associations with COVID-19 incidence and lethality in Madrid under different synoptic meteorological patterns. During the analyzed period (1 January 2020-28 February 2021), with one month before each of three COVID-19 waves were recorded anomalous anticyclonic circulations in the mid-troposphere, with positive anomalies of geopotential heights at 500 mb and favorable stability conditions for SARS-CoV-2 fast diffusion. In addition, the results reveal that air temperature, Planetary Boundary Layer height, ground level ozone have a significant negative relationship with daily new COVID-19 confirmed cases and deaths. The findings of this study provide useful information to the public health authorities and policymakers for optimizing interventions during pandemics.